Potassium isotope heterogeneity in the early Solar System controlled by extensive evaporation and partial recondensation
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Potassium isotope heterogeneity in the early Solar System controlled by extensive evaporation and partial recondensation. / Hu, Yan; Moynier, Frédéric; Bizzarro, Martin.
In: Nature Communications, Vol. 13, 7669, 2022.Research output: Contribution to journal › Journal article › Research › peer-review
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T1 - Potassium isotope heterogeneity in the early Solar System controlled by extensive evaporation and partial recondensation
AU - Hu, Yan
AU - Moynier, Frédéric
AU - Bizzarro, Martin
N1 - Publisher Copyright: © 2022, The Author(s).
PY - 2022
Y1 - 2022
N2 - Volatiles are vital ingredients for a habitable planet. Angrite meteorites sample the most volatile-depleted planetesimal in the Solar System, particularly for the alkali elements. They are prime targets for investigating the formation of volatile-poor rocky planets, yet their exceptionally low volatile content presents a major analytical challenge. Here, we leverage improved sensitivity and precision of K isotopic analysis to constrain the mechanism of extreme K depletion (>99.8%) in angrites. In contrast with the isotopically heavy Moon and Vesta, we find that angrites are strikingly depleted in the heavier K isotopes, which is best explained by partial recondensation of vaporized K following extensive evaporation on the angrite parent body (APB) during magma-ocean stage. Therefore, the APB may provide a rare example of isotope fractionation controlled by condensation, rather than evaporation, at a planetary scale. Furthermore, nebula-wide K isotopic variations primarily reflect volatility-driven fractionations instead of presolar nucleosynthetic heterogeneity proposed previously.
AB - Volatiles are vital ingredients for a habitable planet. Angrite meteorites sample the most volatile-depleted planetesimal in the Solar System, particularly for the alkali elements. They are prime targets for investigating the formation of volatile-poor rocky planets, yet their exceptionally low volatile content presents a major analytical challenge. Here, we leverage improved sensitivity and precision of K isotopic analysis to constrain the mechanism of extreme K depletion (>99.8%) in angrites. In contrast with the isotopically heavy Moon and Vesta, we find that angrites are strikingly depleted in the heavier K isotopes, which is best explained by partial recondensation of vaporized K following extensive evaporation on the angrite parent body (APB) during magma-ocean stage. Therefore, the APB may provide a rare example of isotope fractionation controlled by condensation, rather than evaporation, at a planetary scale. Furthermore, nebula-wide K isotopic variations primarily reflect volatility-driven fractionations instead of presolar nucleosynthetic heterogeneity proposed previously.
U2 - 10.1038/s41467-022-35362-7
DO - 10.1038/s41467-022-35362-7
M3 - Journal article
C2 - 36509778
AN - SCOPUS:85143992862
VL - 13
JO - Nature Communications
JF - Nature Communications
SN - 2041-1723
M1 - 7669
ER -
ID: 335421179